I have a report with a chart containing some bars. They represent values from an underlying query. Now, I would like to place some more values, which are closely related to the first values, inside the bars like this:

Can I do that?
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Not exactly, but you can achieve a similar effect:
From the Series Label Properties dialog, in the General tab change the Label Data to be the new value that you want to appear inside the bar.
If you now preview the report, your new value should appear inside the bars and the existing value should appear on top of them.