I’m interested in using an “unrolled linked list” in my C# application.
Is anyone aware of a stable implementation, especially one that will allow me to configure how much padding to allocate per array?

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According to the 2nd comment in your own link, such a list should be implemented in BigList in the PowerCollections library. It’s open source, so you could have a look at the code and see if it allows for your scenario, or if it can be adapted to fit your needs easily.
Other than that, I am now aware of any .NET implementations you could use.